There is growing interest in the novel concept of operating Enhanced Geothermal Systems (EGS) with CO2 instead of water as heat transmission fluid. Initial studies have suggested that CO2 will achieve larger rates of heat extraction, and can offer geologic storage of carbon as an ancillary benefit. Fluid-rock interactions in EGS operated with CO2 are expected to be vastly different in zones with an aqueous phase present, as compared to the central reservoir zone with anhydrous supercritical CO2. Our numerical simulations of chemically reactive transport show a combination of mineral dissolution and precipitation effects in the peripheral zone of the systems. These could impact reservoir growth and longevity, with important ramifications for sustaining energy recovery, for estimating CO2 loss rates, and for figuring tradeoffs between power generation and geologic storage of CO2.

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